Sisal fiber reinforced high density polyethylene pre-preg for potential application in filament winding

A thermoplastic-penetrated natural fiber belt was developed for potential application in filament winding. Discontinuous sisal fiber bundles were impregnated with high density polyethylene and then connected into continuous pre-pregs via hot-pressing. The interfacial bonding was improved by treating the fibers with sodium hydroxide (NaOH) and three types of coupling agents (NH2C3H6Si(OC2H5)3, C2H3Si(OC2H5)3 and C51H112O22P6Ti). Tensile properties of the fiber bundles, pre-pregs, and annular specimens were determined. The fiber surface microstructure and the pre-preg interfacial bonding were evaluated via scanning electron microscopy and Fourier transform infrared spectroscopy. Among the four treatments, 2% C2H3Si(OC2H5)3 yielded the most significant improvement in the tensile properties of the pre-pregs and annular specimens. The fiber bundle was less damaged by the coupling agents treatment comparing to NaOH treatment. When the overlap at the end of the sisal fibers was >11 mm, the presence of the joint had no effect on the tensile strength of the pre-preg. The pre-preg belt containing treated fibers, which was evaluated based on the requirements of filament winding applications, exhibited a high performance.