Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
11016612 | Fuel | 2019 | 10 Pages |
Abstract
High purity H2 production from shale gas using sorption enhanced chemical looping steam reforming (SE-CLSR) was investigated at 1â¯bar, GHSV 0.498â¯hâ1, feed molar steam to carbon ratio of 3 and 650â¯Â°C for 20 reduction-oxidation-calcination cycles using CaO and 18â¯wt% NiO on Al2O3 as sorbent and catalyst/oxygen carrier (OC) respectively. The shale gas feedstock was able to cyclically reduce the oxygen carrier and subsequently reform with high H2 yield and purity. For example H2 yield of 31â¯wt% of fuel feed and purity of 92% were obtained in the 4th cycle during the pre-breakthrough period (prior to cycles with low sorbent capacity). This was equivalent to 80 and 43% enhancement compared to the conventional steam reforming process respectively.
Related Topics
Physical Sciences and Engineering
Chemical Engineering
Chemical Engineering (General)
Authors
Zainab Ibrahim S G Adiya, Valerie Dupont, Tariq Mahmud,