Article ID Journal Published Year Pages File Type
1263984 Organic Electronics 2013 7 Pages PDF
Abstract

We demonstrate flexible organic light-emitting diodes (FOLEDs) that use flexible conductive polymer electrodes patterned by negative mold transfer printing (nMTP). Because pristine poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) is unsuitable for nMTP owing to problems with wettability, additives are used to improve the surface wetting properties of the polymer on the mold to successfully employ nMTP. Moreover, the additives improve the conductivity of the polymer electrode. FOLEDs fabricated with the modified PEDOT:PSS using nMTP exhibit electrical properties comparable to those of a device having an indium tin oxide (ITO) anode. These results show that the highly conductive PEDOT:PSS patterned by nMTP can be used as transparent high-resolution electrodes in low-cost ITO-free FOLEDs.

Graphical abstractFigure optionsDownload full-size imageDownload as PowerPoint slideHighlights► We present the first demonstration of the nMTP for the flexible OLEDs anode. ► Additives improve the wetting properties and electrical characteristics of PEDOT. ► The conductivity enhancement mechanism can explain with changed PEDOT:PSS. ► A modified polymer electrode showed outstanding resistance stability and flexibility. ► The P-OLEDs exhibited higher EL characteristics more than I-OLED at low current density.

Related Topics
Physical Sciences and Engineering Chemistry Chemistry (General)
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