Alpha self-irradiation effects in ternary oxides of actinides elements: The zircon-like phases AmIIIVO4 and AIINpIV(VO4)2 (A=Sr, Pb)

We report the experimental studies of irradiation damage from alpha decay in neptunium and americium vanadates versus cumulative dose. The isotopes used were the transuranium αα-emitter 237Np and the α,γα,γ-emitter 241Am. Neptunium and americium vanadates self-irradiation was studied by X-ray diffraction method (XRD). The comparison of the powder diffraction patterns reveal that the irradiation has no apparent effect on the neptunium phases while the americium vanadate swells and becomes metamict as a function of cumulative dose.

Graphical abstractWe report the experimental studies of irradiation damage from alpha decay in neptunium and americium vanadates versus cumulative dose. The americium vanadate swells and becomes metamict as a function of cumulative dose.Figure optionsDownload full-size imageDownload as PowerPoint slide