Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
1504114 | Solid State Sciences | 2015 | 5 Pages |
•Large area graphene was successfully synthesized via CVD techniques.•The layers of graphene can be confirmed from HRTEM images.•Homogenous distribution of TiO2 nanoparticles were observed.•Enhanced hydrogen evolution was found from aqueous solution by using sacrificial reagents.
This study reports that the atmospheric pressure chemical vapor deposition (CVD) growth of large area graphene (LAG) over a Cu foil. The obtained large area graphene was further decorated with TiO2 nanoparticles via ultrasonic method. The surface structure, crystal phase, and elemental identification of these obtained LAG/TiO2 composite were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), energy dispersive X-ray (EDX) analysis, and Raman spectra. The photocatalytic H2 evolution result illustrates Cu-LAG/TiO2 has been found to be a potential catalyst for conversion of solar energy to clean hydrogen energy under visible light-driven despite that the H2 evolution activity is not high enough in this stage.
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