Article ID Journal Published Year Pages File Type
1595136 Solid State Communications 2008 5 Pages PDF
Abstract

Transport and magnetic properties of ferromagnetic (FM) insulating La0.875Ca0.125MnO3 (LCMO) manganite have been reported. Temperature variation of field cooled (FC) magnetization shows paramagnetic to ferromagnetic (PM–FM) transition at 168 K (TC)(TC) while ac susceptibility exhibits an additional cusp like downfall around 115 K (TfTf), which shifts with frequency indicating a frustrated magnetic state. Resistivity shows insulating behaviour with a distinct inflection near TCTC. The Shklovskii–Efros (S–E) type variable range hopping mechanism is seen to govern the conduction within the temperature range 156–282 K. Thermoelectric power (TEP) exhibits a peak at ∼TC∼TC and the field dependant resistivity shows different curvatures above and below TCTC. Such behaviours suggest that the PM–FM transition is mediated by double exchange (DE) mechanism similar to that observed in FM metallic manganites. Unexpectedly, magnetoresistance data analysis shows that DE mechanism persists in this sample even down to 50 K. Thus the DE mechanism plays an important role even in case of ferromagnetic insulating manganite La0.875Ca0.125MnO3, governing the magnetic and electrical properties.

Related Topics
Physical Sciences and Engineering Materials Science Materials Science (General)
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