Article ID Journal Published Year Pages File Type
1667002 Thin Solid Films 2012 6 Pages PDF
Abstract

A simple process is described for directly synthesizing pure graphene and N-doped graphene sheets from ethanol flame and amine plus ethanol flames respectively. The microstructures and nitrogen contents of the graphenes were characterized using scanning and transmission electron spectroscopy, X-ray photoelectron spectroscopy and Raman spectroscopy. The results reveal that: (1) The graphene sheets from flame exhibit good transparency and a large size up to 400 μm2 with few layers and folded edges; (2) The nitrogen-doped graphene sheets have a dominant ‘pyridine-type’ structure with CN bonds (one N atom bonded to two C atoms); (3) Compared with other methods, the graphene sheets from flame have more surface defects due to the environmental conditions and introduction of nitrogen atoms, which makes it a promising material for supercapacitors and catalyst supports.

► Synthesis of graphene and nitrogen doped graphene from flame. ► Graphene sheets from flame exhibited a good transparency and a large size. ► Graphene from flame had more surface defects due to environmental conditions.

Related Topics
Physical Sciences and Engineering Materials Science Nanotechnology
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