Article ID Journal Published Year Pages File Type
1739138 Journal of Environmental Radioactivity 2008 5 Pages PDF
Abstract

137Cs is an artificial radionuclide with a half-life of 30.12 years which released into the environment as a result of atmospheric testing of thermo-nuclear weapons primarily during the period of 1950sā€“1970s with the maximum rate of 137Cs fallout from atmosphere in 1963. 137Cs fallout is strongly and rapidly adsorbed by fine particles in the surface horizons of the soil, when it falls down on the ground mostly with precipitation. Its subsequent redistribution is associated with movements of the soil or sediment particles. The 137Cs nuclide tracing technique has been used for assessment of soil losses for both undisturbed and cultivated soils. For undisturbed soils, a simple profile-shape model was developed in 1990 to describe the 137Cs depth distribution in profile, where the maximum 137Cs occurs in the surface horizon and it exponentially decreases with depth. The model implied that the total 137Cs fallout amount deposited on the earth surface in 1963 and the 137Cs profile shape has not changed with time. The model has been widely used for assessment of soil losses on undisturbed land.However, temporal variations of 137Cs depth distribution in undisturbed soils after its deposition on the ground due to downward transport processes are not considered in the previous simple profile-shape model. Thus, the soil losses are overestimated by the model. On the base of the erosion assessment model developed by Walling, D.E., He, Q. [1999. Improved models for estimating soil erosion rates from cesium-137 measurements. Journal of Environmental Quality 28, 611ā€“622], we discuss the 137Cs transport process in the eroded soil profile and make some simplification to the model, develop a method to estimate the soil erosion rate more expediently. To compare the soil erosion rates calculated by the simple profile-shape model and the simple transport model, the soil losses related to different 137Cs loss proportions of the reference inventory at the Kaixian site of the Three Gorge Region, China are estimated by the two models. The over-estimation of the soil loss by using the previous simple profile-shape model obviously increases with the time period from the sampling year to the year of 1963 and 137Cs loss proportion of the reference inventory. As to 20ā€“80% of 137Cs loss proportions of the reference inventory at the Kaixian site in 2004, the annual soil loss depths estimated by the new simplified transport process model are only 57.90ā€“56.24% of the values estimated by the previous model.

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Physical Sciences and Engineering Energy Nuclear Energy and Engineering
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