Transient magnetoviscosity of dilute ferrofluids

The magnetic field induced change in the viscosity of a ferrofluid, commonly known as the magnetoviscous effect and parameterized through the magnetoviscosity, is one of the most interesting and practically relevant aspects of ferrofluid phenomena. Although the steady state behavior of ferrofluids under conditions of applied constant magnetic fields has received considerable attention, comparatively little attention has been given to the transient response of the magnetoviscosity to changes in the applied magnetic field or rate of shear deformation. Such transient response can provide further insight into the dynamics of ferrofluids and find practical application in the design of devices that take advantage of the magnetoviscous effect and inevitably must deal with changes in the applied magnetic field and deformation. In this contribution Brownian dynamics simulations and a simple model based on the ferrohydrodynamics equations are applied to explore the dependence of the transient magnetoviscosity for two cases: (I) a ferrofluid in a constant shear flow wherein the magnetic field is suddenly turned on, and (II) a ferrofluid in a constant magnetic field wherein the shear flow is suddenly started. Both simulations and analysis show that the transient approach to a steady state magnetoviscosity can be either monotonic or oscillatory depending on the relative magnitudes of the applied magnetic field and shear rate.

Research Highlights►Rotational Brownian dynamics simulations were used to study the transient behavior of the magnetoviscosity of ferrofluids. ►Damped and oscillatory approach to steady state magnetoviscosity was observed for step changes in shear rate and magnetic field. ►A model based on the ferrohydrodynamics equations qualitatively captured the damped and oscillatory features of the transient response ►The transient behavior is due to the interplay of hydrodynamic, magnetic, and Brownian torques on the suspended particles.