Stress relaxation in Fe/Si neutron supermirrors by He+ irradiation

Magnetic supermirrors are widely used in polarized neutron applications. A key issue in producing these multilayer structures is to avoid residual stress in the layers, which may cause the layers to peel off. In this work He+ ion irradiation of 500 keV energy was applied at fluences of 1, 24, 50, 100×1014 ions/cm2 with the aim of reducing residual stress. Structural, magnetic and neutron-optical properties were investigated by grazing incidence high-angle X-ray diffraction, magneto-optical Kerr effect, conversion electron Mössbauer spectroscopy and polarized neutron reflectometry. We find a monotonous decrease of the tensile stress upon irradiation from 1.76 to 0.37 GPa with a coupled decrease of neutron reflectivity at the critical angle and decrease of the maximum polarizing efficiency from 23% to 4% at the highest fluence compared to the as-prepared reference supermirror. The supermirrors exhibit a superposition of uniaxial and fourfold in-plane magnetic anisotropy.