Magnetization and heat capacity studies of double perovskite compounds Ba2SmRuO6 and Ba2DyRuO6

Here we report the magnetic and heat capacity studies of the double perovskite compounds Ba2SmRuO6 and Ba2DyRuO6. Antiferromagnetic transitions are inferred at 54 and 47 K in Ba2SmRuO6 and Ba2DyRuO6, respectively, in the magnetization measurements. Heat capacity measurements show large jumps at the corresponding temperatures and confirm the bulk magnetic ordering. Both the measurements provide clear indication of the ordering of the rare earth moments also along with the Ruthenium moments. However, the heat capacity results suggest that the ordering of rare earth magnetic moments is spread over a large temperature range. An anomaly observed in the magnetization measurements at 42 K (below the magnetic ordering) in Ba2SmRuO6 is discerned as a reorientation of Sm3+ moments.