Structural and magnetic properties of Fe1+dTe single crystals

We have grown single crystals of Fe1+dTe by a conventional self-flux method. We obtained plate-like single crystals with dnom ≥ 0.1. The value of the magnetization increased with increasing excess Fe concentration, and a broadening of the antiferromagnetic transition was observed for dnom >1.15. Further, we noted that the antiferromagnetic transition of Fe1.134Te (dnom = 0.15) was clearly suppressed to a lower temperature, which would indicate a possibility of controllability of magnetism by excess Fe concentration.