Article ID Journal Published Year Pages File Type
209402 Fuel Processing Technology 2015 6 Pages PDF
Abstract

•A pilot plant for CO2 capture was tested with K2CO3 solvent promoted with glycine.•Addition of 10 wt.% glycine was found to improve the CO2 recovery rate by up to 6 times.•Pressure drop, holdup and CO2 removal efficiency for the absorber were presented.•Absorber performance data was used to validate an Aspen Plus simulation.

The absorption performance of a glycine promoted precipitating potassium carbonate (K2CO3) solvent absorption process for carbon dioxide (CO2) capture has been presented using a laboratory scale pilot plant. Glycine has been added as a rate promoter to 40–45 wt.% K2CO3 solutions to examine the enhancement of the CO2 absorption process. The laboratory scale pilot plant has been designed to capture 4–10 kg/hr of CO2 from an air/CO2 mixture at a feed gas rate of 30–55 kg/hr. Performance data of the absorber including pressure drop, holdup and CO2 removal efficiency has been collected from the pilot plant and presented for a range of operating conditions. The addition of glycine was found to improve the CO2 recovery rate by up to 6 times whilst also slightly increasing the pressure drop and holdup measured in the packed absorption column which is likely due to a reduction in the surface tension of the solvent. Additionally, increasing the K2CO3 solvent concentration and operating with a higher CO2 feed gas concentration were found to increase the CO2 recovery results. Finally performance data from the absorber has been used to validate an Aspen Plus simulation of the system.

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Physical Sciences and Engineering Chemical Engineering Chemical Engineering (General)
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