Article ID Journal Published Year Pages File Type
4444505 Atmospheric Environment 2006 10 Pages PDF
Abstract

The concentrations of five hazardous air pollutants were simulated using the community multi-scale air quality (CMAQ) modeling system. Annual simulations were performed over the continental United States for the entire year of 2001 to support human exposure estimates. Results are shown for formaldehyde, acetaldehyde, benzene, 1,3-butadiene and acrolein. Photochemical production in the atmosphere is predicted to dominate ambient formaldehyde and acetaldehyde concentrations, and to account for a significant fraction of ambient acrolein concentrations. Spatial and temporal variations are large throughout the domain over the year. Predicted concentrations are compared with observations for formaldehyde, acetaldehyde, benzene and 1,3-butadiene. Although the modeling results indicate an overall slight tendency towards underprediction, they reproduce episodic and seasonal behavior of pollutant concentrations at many monitors with good skill.

Related Topics
Physical Sciences and Engineering Earth and Planetary Sciences Atmospheric Science
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