Article ID Journal Published Year Pages File Type
4450450 Atmospheric Research 2011 13 Pages PDF
Abstract

Wet and dry deposition samples were collected along with the ambient air samples between September 2008 and June 2009 in an urban site, BUTAL, Turkey. A modified deposition sampler was used for dry and wet periods. Average dissolved and particle phase wet deposition flux values were determined to be 7.4 ± 7.3 μg/m2 day and 21 ± 30 μg/m2 day, respectively. The highest PAH wet fluxes were observed in the winter and fall seasons. Dissolved and particle phase rainwater concentrations of PAHs were 290 ng/L and 665 ng/L. The average of total (particle + gas) atmospheric concentration of ∑12PAH was 130 ± 160 ng/m3. In general, percentages of PAHs with five or more aromatic rings were bigger in particle phase in air. Average washout ratios of PAH compounds were determined 8.97 × 105 and 8.52 × 105 for gas and particle phase, respectively. Gas phase washout ratios of high molecular weight PAHs were greater than the lower molecular weight PAHs.

Research highlights► Wet deposition and ambient air concentrations of polyaromatic hydrocarbons (PAHs) were collected at an urban site. ► Gas and particle phase concentrations in air and rainwater were determined. ► Coal combustion was the dominant source for air and rainwater levels in winter. ► Higher molecular weight PAHs had greater washout ratios than the lower ones.

Related Topics
Physical Sciences and Engineering Earth and Planetary Sciences Atmospheric Science
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