Article ID Journal Published Year Pages File Type
46024 Applied Catalysis B: Environmental 2013 10 Pages PDF
Abstract

Microreactors based on Cu, Ce oxides dispersed onto zeolite films grown on brass microgrids were developed. Secondary synthesis conditions were regulated in order to obtain thin, homogeneous and adherent coatings of mordenite to which Cu and Ce were later incorporated. The systems were characterized by XRD, SEM-EPMA, H2-TPR, LRS and XPS. The catalytic coatings were mechanically and chemically stable under reaction. Cu, Ce/zeolite microreactors were evaluated in the CO total oxidation (COTox) and in the preferential CO oxidation (COProx) showing a superior performance when compared with the same powder catalyst.

Graphical abstractFigure optionsDownload full-size imageDownload as PowerPoint slideHighlights► Zeolite-based microreactors for CO oxidation. ► Synthesis of continuous and stable catalytic films on brass microgrids. ► Highly dispersed phases of Cu and Ce on the zeolite-coated microreactors. ► Superior performance in COTox and COProx reactions than powder catalysts.

Related Topics
Physical Sciences and Engineering Chemical Engineering Catalysis
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