Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
49968 | Catalysis Communications | 2012 | 4 Pages |
SnO2–MnOx–CeO2 catalysts prepared by a co-precipitation method have been investigated for NH3-SCR reaction. The catalyst with a molar ratio of Sn / (Sn + Mn + Ce) = 0.1 showed complete conversion of NO in a temperature range of 80–230 °C. A remarkably high activity, N2 selectivity and SO2 resistance was obtained at 200–500 °C, attributed to the significantly enhanced Lewis acid sites that are created by surface sulfation during SO2-containing SCR reaction.
Graphical abstractFigure optionsDownload full-size imageDownload as PowerPoint slideHighlights► The SnO2-MnOx-CeO2 catalyst showed 100% conversion of NO at 80–230°C. ► A remarkably high N2 selectivity and SO2 resistance was obtained at 200–500°C. ► The Lewis acid sites are significantly enhanced by SO2 poisoning in SCR reaction.