Article ID Journal Published Year Pages File Type
5140244 Spectrochimica Acta Part B: Atomic Spectroscopy 2017 14 Pages PDF
Abstract
Multi-parametric theoretical studies to analyze the effect of both the matter properties (absorption coefficient, thermal conductivity and diffusivity) and the heating field parameters (spatial distribution and pulse duration) on the resulted temperature distribution are presented. For heating in sub-micrometric range (< 1 μm), a low dependence of heating temperature distribution on the sample thermal properties and heating source duration was observed. Nano-ablation thresholds are found to be increasing inversely with heating source dimensions. The simulation results demonstrated a good agreement with the nanometer-size craters (100 nm diameters, 10 nm depth) obtained experimentally with a tip-enhanced near-field ablation (4 ns laser pulse duration, 266 nm wavelength) of Si- and Au-samples.
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Physical Sciences and Engineering Chemistry Analytical Chemistry
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