Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
5376627 | Chemical Physics | 2007 | 7 Pages |
Abstract
The vibronic quantum dynamics in molecular dimer systems taking place after the interaction with an ultrashort pulse is studied. Therefore, an established model incorporating a single monomer vibrational degree of freedom and a single exciton coupling is employed. The time-scale for the exciton transfer and internal vibrational dynamics is investigated as a function of the laser pulse parameters. The appearance of pump-probe signals is analyzed in terms of molecular geometry and properties of the external fields.
Related Topics
Physical Sciences and Engineering
Chemistry
Physical and Theoretical Chemistry
Authors
Joachim Seibt, Volker Engel,