Article ID Journal Published Year Pages File Type
5382972 Chemical Physics Letters 2012 7 Pages PDF
Abstract
► Quantum study of matrix response upon femtosecond photoecxitation of NO impurity. ► High-dimensional quantum propagation is performed using the MCTDH method. ► Mean field results overestimate vibrational coherences. ► Correlations lead to small, but measurable effects in simulated pump-probe spectra.
Related Topics
Physical Sciences and Engineering Chemistry Physical and Theoretical Chemistry
Authors
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