Reaction efficiency of diffusion-controlled processes on finite, aperiodic planar lattices - III: Supramolecular architectures

► We study the reaction efficiency of diffusion-controlled processes on surfaces. ► We consider finite, aperiodic planar lattices and supramolecular architectures. ► We consider the irreversible reaction A + B → C on a finite, discretized d = 2 surface. ► A lattice-statistical model is developed to quantify the reaction efficiency. ► Aperiodic or regular surfaces better optimize surficial reactions than Ω = 0 hosts.