Article ID Journal Published Year Pages File Type
5383334 Chemical Physics Letters 2012 5 Pages PDF
Abstract
► We consider non-linear response functions for a simple two-level molecular system. ► It is shown that it cannot be constructed using a single reduced density matrix master equation. ► A set of master equations is derived which together reproduce the two-level response function. ► Parametric projection operators are introduced to derive proper equations in general cases.
Related Topics
Physical Sciences and Engineering Chemistry Physical and Theoretical Chemistry
Preview
Quantum master equations for non-linear optical response of molecular systems
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