Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
5384041 | Chemical Physics Letters | 2011 | 10 Pages |
Abstract
⺠We explain ambiguities in simulations of nonlinear optical surface spectroscopy. ⺠There is an ambiguity in the definition of the electric-dipole-order surface signal. ⺠There is also an ambiguity in the definition of the quadrupole-order bulk signal. ⺠These two ambiguities are equal and opposite, so the total signal is unambiguous. ⺠Our simulations of the water-air interface support this picture.
Related Topics
Physical Sciences and Engineering
Chemistry
Physical and Theoretical Chemistry
Authors
Steven J. Byrnes, Phillip L. Geissler, Y.R. Shen,