Article ID Journal Published Year Pages File Type
5384041 Chemical Physics Letters 2011 10 Pages PDF
Abstract
► We explain ambiguities in simulations of nonlinear optical surface spectroscopy. ► There is an ambiguity in the definition of the electric-dipole-order surface signal. ► There is also an ambiguity in the definition of the quadrupole-order bulk signal. ► These two ambiguities are equal and opposite, so the total signal is unambiguous. ► Our simulations of the water-air interface support this picture.
Related Topics
Physical Sciences and Engineering Chemistry Physical and Theoretical Chemistry
Authors
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