Article ID Journal Published Year Pages File Type
5391071 Chemical Physics Letters 2006 5 Pages PDF
Abstract
Two-body Coulomb explosion processes of methanol (CH3OH) in an intense laser field (0.2 PW/cm2, 60 fs) are investigated by the coincidence momentum imaging method. In the coincidence momentum images, the hydrogen ejection processes, CH3OH2+→Hm++CH(3-m)OH+(m=1-3), are securely identified. From the anisotropy in the angular distributions of the fragment ions, the lifetimes of the corresponding precursor ions CH3OH2+ are estimated to be 70-290 fs for the H+ ejection, 110-550 fs for the H2+ ejection, and much longer than 1.4 ps for the H3+ ejection.
Related Topics
Physical Sciences and Engineering Chemistry Physical and Theoretical Chemistry
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