| Article ID | Journal | Published Year | Pages | File Type |
|---|---|---|---|---|
| 7834989 | Applied Surface Science | 2018 | 34 Pages |
Abstract
A series of MFI zeolites with different Si/Al ratios were pretreated by a basic solution and their catalytic activity was evaluated in N2O decomposition after iron exchange. The performance of Fe-ZSM-5 catalysts could be improved by alkaline pretreatment. Among these samples, the activity curve of Fe-Z5-250-S sample could move to low temperature by >100â¯Â°C with a good preservation of hydrothermal stability. It is found that with the meso-microporous hybrid structure, the content of iron as active metal is significantly increased. Additionally, well preservation of the chemical environment around the tetrahedral aluminum and the site accessibility probably may be the other important factors to influence the catalytic activity.
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Authors
Qun Shen, Minfang Wu, Hui Wang, Nannan Sun, Chi He, Wei Wei,