Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
7839259 | Journal of Electron Spectroscopy and Related Phenomena | 2018 | 27 Pages |
Abstract
A theoretical study has been conducted on nondipole asymmetry parameters and angular distribution of Kr 1s1/2 and 4p3/2 photoelectrons with Dirac-Fock method based on the density matrix theory, with a focus on the impacts of nondipoles on the photoelectron angular distribution. The results show that the electric-dipole-electric-quadrupole E1 and E2 interference has a significant influence on the spatial angular distribution of Kr 1s1/2 and 4p3/2 photoelectrons. To be specific, the photoelectron characteristics relevant to the direction of the polarization vector of the incident light can be destroyed by the E1 and E2 interference. For the Kr 4p3/2 photoelectron, it is suggested that the non-dipole effects of photoelectron distribution be measured in two energy positions where the electric dipole β parameter equals to zero. Higher order nondipole effects are negligible according to the investigations. Our calculations consist well with the available experimental and theoretical results.
Keywords
Related Topics
Physical Sciences and Engineering
Chemistry
Physical and Theoretical Chemistry
Authors
Kun Ma, Zhan-Bin Chen, Lu-You Xie, Xiao-Bin Ding, Deng-Hong Zhang, Chen-Zhong Dong,