Article ID Journal Published Year Pages File Type
9586196 Journal of Luminescence 2005 5 Pages PDF
Abstract
High spatial localization of an optical near field allows us to access and excite individual nanometric materials that are much smaller than the diffraction limit of light, while propagating or far-field light can only excite the system globally. This difference, as an initial condition, provides the new exciton dynamics by effective use of a dark state, or a dipole-forbidden state in a quantum-dot (QD) system coupled by the optical near field. We show theoretically and experimentally excitation energy transfer between CuCl quantum cubes, using temporally and spatially resolved near-field spectroscopy. In addition, we report another new feature of the exciton dynamics inherent in a similar system, or characteristic functional (AND/XOR-logic) operations, depending on the initial excitation as well as symmetry of the spatial arrangement of the QDs.
Related Topics
Physical Sciences and Engineering Chemistry Physical and Theoretical Chemistry
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