Article ID Journal Published Year Pages File Type
1180904 Chemometrics and Intelligent Laboratory Systems 2014 8 Pages PDF
Abstract

•A compact formulation of the tri-linear PLS2 procedure was proposed.•Equivalence to tri-linear PLS2 was demonstrated.•Convergence criteria were proved.

This paper focuses on multi-way PLS for discrimination. Emphasis was placed on the computation of parameters (so-called scores and loadings) using an iterative procedure called tri-linear PLS2. In the context of discrimination, this algorithm is applied to a dummy matrix representing group membership, and according to its specific formalism, the tri-linear PLS2 procedure offers the possibility of simplification. The purpose of this paper is to introduce a compact formulation of the tri-linear PLS2 procedure adapted for a discrimination setting. A property of this variant that allows formally establishing its convergence and, by extension, the convergence of the tri-linear PLS2 will be demonstrated. The potential of this compact form will be illustrated with simulated examples.

Related Topics
Physical Sciences and Engineering Chemistry Analytical Chemistry
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