Article ID Journal Published Year Pages File Type
1276296 International Journal of Hydrogen Energy 2012 11 Pages PDF
Abstract

The feasibility of using sintered stainless steel fiber felt (SSSFF) as gas diffusion layer (GDL) in proton exchange membrane fuel cells (PEMFCs) is evaluated in this study. The SSSFF is coated with an amorphous carbon (a-C) film by closed field unbalanced magnetron sputter ion plating (CFUBMSIP) to enhance the corrosion resistance and reduce the contact resistance. The characteristics of treated SSSFF, including microscopic morphology, mechanical properties, electrical conductivity, electrochemical behavior and wettablity characterization, are systematically investigated and summarized according to the requirements of GDL in PEMFC. A membrane electrode assembly (MEA) with a-C coated SSSFF-15 GDL is fabricated and assembled with a-C coated stainless steel bipolar plates in a single cell. The initial peak power density of the single cell is 877.8 mW cm−2 at a current density of 2324.9 mA cm−2. Lifetime test of the single cell over 200 h indicates that the a-C coating protects the SSSFF-15 GDL from corrosion and decreases the performance degradation from 30.6% to 6.3%. The results show that the SSSFF GDL, enjoying higher compressive modulus and ductility, is a promising solution to improve fluid permeability of GDL under compression and PEMFC durability.

► The compressive modulus and ductility of GDL were improved by a novel porous metal of sintered stainless steel fiber felt(SSSFF). ► The corrosion resistance of metal GDL was enhanced and the contact resistance was reduced using amorphous carbon(a-C) coating. ► The key characteristics of treated SSSFF were comparable to carbon paper GDL. ► PEMFC tests showed good initial and lifetime performance on the single cell assembled with a-C coated SSSFF GDL.

Related Topics
Physical Sciences and Engineering Chemistry Electrochemistry
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