Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
1280339 | International Journal of Hydrogen Energy | 2007 | 8 Pages |
The operating performance of a bubbling fluidized-bed membrane reactor for generating hydrogen was investigated using Pd–Ag planar membranes and both a steam methane reforming (SMR) catalyst and an autothermal reforming (ATR) catalyst. The reactor was mostly operated at 500–600∘C and 1500–2600 kPa. A detailed parametric study showed improved overall membrane effectiveness factors and hydrogen permeation fluxes compared with previous tests. Hydrogen permeation fluxes were 4.8–12Nm3/m2h for SMR catalyst operations and 9–18Nm3/m2h for ATR catalyst operations, significantly higher than previous hydrogen permeation fluxes reported in the literature. The ATR catalyst led to better performance than the SMR catalyst. Some catalyst particles were lost during operation with both catalysts, while the catalyst activity was stable.