Article ID Journal Published Year Pages File Type
1285306 Journal of Power Sources 2016 9 Pages PDF
Abstract

•Detection of microstructure with synchrotron X-ray tomography.•Mechanical compression of the microstructure.•Virtual compression of a stochastic geometry model.•Transport simulation with the Lattice Boltzmann method.

Gas transport in non-woven gas diffusion layers of a high-temperature polymer electrolyte fuel cell was calculated with the Lattice Boltzmann method. The underlying micro structure was taken from two sources. A real micro structure was analyzed in the synchrotron under the impact of a compression mask mimicking the channel/rib structure of a flow field. Furthermore a stochastic geometry model based on synchrotron X-ray tomography studies was applied. The effect of compression is included in the stochastic model. Gas transport in these micro structures was simulated and the impact of compression was analyzed. Fiber bundles overlaying the micro structure were identified which affect the homogeneity of the gas flow. There are significant deviations between the impact of compression on effective material properties for this type of gas diffusion layers and the Kozeny-Carman equation.

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Related Topics
Physical Sciences and Engineering Chemistry Electrochemistry
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