Article ID | Journal | Published Year | Pages | File Type |
---|---|---|---|---|
4762985 | Chemical Engineering Journal | 2017 | 52 Pages |
Abstract
The total operation pressure (from 1 to 9 bar) did not have an important influence on H2 yield, and/or materials performance. Sorbent carbonation reaction rates up to 4.42 * 10â2 kmol hâ1 kg sorbâ1 were determined in the experiments, being this parameter responsible of the limit in CH4 space velocity that can be successfully converted through this sorbent/catalyst system. The experimental results have been successfully described by a pseudo-homogeneous reactor model that incorporates the main kinetic expressions of the reactions involved in the SER stage.
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Authors
G. Grasa, M.V. Navarro, J.M. López, L. DÃez-MartÃn, J.R. Fernández, R. Murillo,