کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
4996345 | 1459794 | 2017 | 9 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Organosolv extraction of softwood combined with lignin-to-liquid-solvolysis as a semi-continuous percolation reactor
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی شیمی
تکنولوژی و شیمی فرآیندی
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
As part of a concept for a continuous biorefining process, a fractionation procedure for lignocellulosic biomass based on flow-through organosolv lignin solubilisation has been developed and tested. Lignin is removed from the biomass in a continuous flow-through system, producing a dissolved lignin fraction and a residual fibre fraction rich in cellulose. A solvent system comprising ethanol, water and sulfuric or formic acid as catalyst is tested over a 413-468Â K temperature range. Process conditions that are suitable for fractionation of softwood from Norway spruce are determined using an experimental design. The best conditions give yields up to 86% of the initially determined lignin mass, leaving a clean fibre residue that corresponds to 67% of the initial cellulose mass. The produced lignin fraction can be converted by formic acid assisted solvolysis to a liquid comprising mostly methoxy-phenols at nearly 90% mass yield. The results show that the continuous flow fractionation of lignocellulosic biomass is a promising route for biorefinery processing.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Biomass and Bioenergy - Volume 99, April 2017, Pages 147-155
Journal: Biomass and Bioenergy - Volume 99, April 2017, Pages 147-155
نویسندگان
Camilla Løhre, Mike Kleinert, Tanja Barth,