کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
5349593 | 1503644 | 2014 | 11 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Amidoxime-grafted multiwalled carbon nanotubes by plasma techniques for efficient removal of uranium(VI)
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
شیمی تئوریک و عملی
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
A novel solid-phase extractant, amidoxime-grafted multiwalled carbon nanotubes (AO-g-MWCNTs), has been synthesized using plasma techniques to selectively separate uranium from nuclear industrial effluents. The adsorbent was characterized by Fourier transform infrared spectra (FT-IR), elemental analysis, Raman, scanning electron microscopy (SEM), and thermal gravity analysis (TGA). Sorption behaviors of uranium(VI) on AO-g-MWCNTs were investigated by varying pH, contact time, initial uranium concentration, and temperature. An optimum sorption capacity of 145 mg gâ1 (0.61 mmol gâ1) for U(VI) was obtained at pH 4.5. X-ray photoelectron spectroscopy (XPS) has been used to explore the sorption mechanism of U(VI) on AO-g-MWCNTs. Furthermore, AO-g-MWCNTs could selectively adsorb U(VI) in aqueous solution containing co-existing ions (Mn2+, Co2+, Ni2+, Zn2+, Sr2+, Ba2+ and Cs+). This study shows that AO-g-MWCNTs are potential adsorbent for effective removal of U(VI) from aqueous solution.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Applied Surface Science - Volume 320, 30 November 2014, Pages 10-20
Journal: Applied Surface Science - Volume 320, 30 November 2014, Pages 10-20
نویسندگان
Yun Wang, Zexing Gu, Jijun Yang, Jiali Liao, Yuanyou Yang, Ning Liu, Jun Tang,