کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
621136 1455160 2016 10 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
Influence of mixing on particle formation of fast precipitation reactions—A new coarse graining method using CFD calculations as a “measuring” instrument
ترجمه فارسی عنوان
اثر اختلاط بر شکل گیری ذرات واکنش های بارش سریع؛ روش جدید graining درشت با استفاده از محاسبات CFD به عنوان یک ابزار "اندازه گیری"
کلمات کلیدی
بارش؛ معادله تعادل جمعیت؛ میکسر جت برخورد محدود ؛ مخلوط کردن؛ روش STAR NM ؛ روش graining درشت
موضوعات مرتبط
مهندسی و علوم پایه مهندسی شیمی تصفیه و جداسازی
چکیده انگلیسی


• A new CFD coarse graining approach called STAR NM is presented.
• STAR NM means “Spatially and Temporally Averaged Reduced Numeric Measurement”.
• The method presented demonstrates how to deviate short-cut models from CFD.
• The influence of mixing on the particle formation at precipitation is investigated.
• Comparison of simulated particle size distributions to experiments is made.

Methods based on Computational Fluid Dynamics (CFD) are a promising tool to gain insight into poorly accessible and swift solid formation processes such as granulation or precipitation. Unfortunately, CFD modeling of transient particle size distributions in such reactors requires enormous computational effort because complex and multi-scale interactions have to be considered. Hence, a new coarse graining approach is presented with which these complex interactions can be handled with reasonable computational effort and which enables to extract short cut methods from complex CFD simulations.The method is exemplified for precipitation crystallization of nanoscaled solid particles from the liquid phase. This process is governed by fast primary processes, such as supersaturation build-up, nucleation and growth. Experimental access to internal parameters is very difficult or even impossible.The new methodology which we call “Spatially and Temporally Averaged Reduced Numeric Measurement” (STAR NM) is based on a reasonable averaging and correlation of process dominating state variables or rates which are consigned to a fast 1D population balance solver. Precipitation of the sparingly soluble barium sulfate in water is used as a model process. A confined impinging jet mixer is used as a benchmark apparatus which allows for the adjustment of highly reproducible mixing conditions. Experimental results are compared to those gained with the new STAR NM approach.

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ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Chemical Engineering Research and Design - Volume 108, April 2016, Pages 176–185
نویسندگان
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