کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
10262683 457058 2006 11 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
Validation of bubble breakage, coalescence and mass transfer models for gas-liquid dispersion in agitated vessel
موضوعات مرتبط
مهندسی و علوم پایه مهندسی شیمی مهندسی شیمی (عمومی)
پیش نمایش صفحه اول مقاله
Validation of bubble breakage, coalescence and mass transfer models for gas-liquid dispersion in agitated vessel
چکیده انگلیسی
A multiblock stirred tank model with discretized population balances for bubbles and two-film Maxwell-Stefan multicomponent mass transfer between gas and liquid was created for the 194dm3 agitated vessel. The model considers local mass transfer conditions in the vessel and is simple enough for the mathematical optimization of unknown model parameters. Unknown parameters in the mechanistic bubble breakage and coalescence models were fitted against measured local BSDs. After this, a parameter in the liquid film mass transfer correlation was adjusted against absorption and desorption experiments of oxygen. Local gas-liquid mass transfer areas were calculated from the population balance model. The simulations with the validated models show good agreement against experiments. On the other hand, the fitted parameters deviate from the theoretical values, which emphasizes the need of model validation against accurate experiments. Due to their fundamental character and the validation process, the fitted models seem to be useful tools for the design and scale-up of agitated gas-liquid reactors.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Chemical Engineering Science - Volume 61, Issue 1, January 2006, Pages 218-228
نویسندگان
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