کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
11000849 | 1428062 | 2018 | 11 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Two-train elevated-temperature pressure swing adsorption for high-purity hydrogen production
ترجمه فارسی عنوان
جذب نوسان فشار بر دو قطار برای تولید هیدروژن خلوص بالا
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کلمات کلیدی
جذب نوسان فشار دمای بالا، اکسید دو لایه لایه ای پتاسیم، تولید هیدروژن، گاز منتقل شده،
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی انرژی
مهندسی انرژی و فناوری های برق
چکیده انگلیسی
The trade-off between hydrogen recovery ratio (HRR) and hydrogen purity (HP) is one of the main drawbacks in normal temperature pressure swing adsorption (NT-PSA) for producing high-purity hydrogen from shifted gas. In this paper, a two-train elevated-temperature pressure swing adsorption (ET-PSA) process that achieved 99.999% HP and over 95% HRR is proposed, which has wide application potentials in fuel cells and chemical industries. Potassium-promoted layered double oxide (K-LDO), which shows reasonable working capacity and fast adsorption/desorption kinetics at elevated temperatures (200-450â¯Â°C), is adopted as the CO2 adsorbent. CO in the shifted gas is co-purified by high-temperature water gas shift (WGS) catalysts added to the columns. The first-train ET-PSA adopted an eight-column thirteen-step configuration with shorter step time to remove most of the CO/CO2 in the shifted gas, and the second-train ET-PSA adopted a double-column seven-step configuration with longer step time to purify the residual gas impurities. The introduction of co-current high-pressure steam rinse and counter-current low-pressure steam purge is the key to achieve both high HRR and HP. The high-temperature steam is the main energy consumption of ET-PSA rather than low HRR in NT-PSA, and the total steam consumption is reduced by adopting the tail gas from second-train ET-PSA as the purge gas for first-train ET-PSA. The optimal results achieved 97.51% HRR and 99.9994% HP with only 0.188 rinse-to-feed ratio and 0.263 purge-to-feed ratio, which are the highest values reported for PSAs producing high-purity hydrogen from carbon-based fuels.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Applied Energy - Volume 229, 1 November 2018, Pages 1061-1071
Journal: Applied Energy - Volume 229, 1 November 2018, Pages 1061-1071
نویسندگان
Xuancan Zhu, Yixiang Shi, Shuang Li, Ningsheng Cai,