کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
1888036 | 1533400 | 2016 | 4 صفحه PDF | دانلود رایگان |
• Distribution of secondary electrons thermalization length is calculated for LaPO4 and LuPO4.
• Dependence of X-ray excited luminescence intensity on the nanoparticle size was simulated.
• Correlation of experimental and simulated dependencies was found.
• The search criteria for scintillating nanoparticles is proposed.
The thermalization length distribution of electrons over their kinetic energy in a conduction band is calculated on the basis of the data on the electron effective mass, density of states in conduction band, dielectric permittivity and energy of longitudinal optical phonons. The method of modeling of a recombinational luminescence intensity dependence on the nanoparticle size is proposed on the basis of the assumption that the contribution to a recombinational luminescence gives only those charge carriers which in the result of thermalization did not reach a near-surface layer of nanoparticles. Using such the approach the theoretical dependence of recombinational luminescence intensity on the nanoparticle size for LaPO4 and LuPO4 are calculated. The revealed correlation of experimental and theoretical dependences confirms that the commensurability of electron thermalization length with nanoparticle size is the main reason of the sharp decrease of X-ray excited luminescence intensity when the nanoparticle size decreases.
Journal: Radiation Measurements - Volume 90, July 2016, Pages 174–177