T-matrix approach to calculating circular polarization of aggregates made of optically active materials

Optical activity is a typical property of the biological materials where left-handed amino-acids and right-handed carbohydrates dominate (so called homochirality). Observationally, optically active materials reveal themselves through the circular polarization in the light they scatter. Thus, circular polarization produced by the optically active particles can serve as a biomarker. It is known that biological (e.g. colonies of bacteria) and pre-biological (e.g. dust in comets) particles often have a complex structure that can be modeled presenting them as aggregates of small monomers. This motivated the development of the T-matrix code presented in this paper, which enables calculation of the scattering matrix - including circular polarization - of the light scattered by aggregated optically active particles. The code can be used for modeling the light scattering by biological objects (e.g. colonies of bacteria, blood cells) and for interpretation of the circular polarization produced by the cosmic dust that contains (pre)biological organic, e.g. comet dust or planetary aerosols.

Research highlights► The multiple sphere T-matrix method is extended to optically active (OA) spheres. ► A code for implementation of the formulation is described. ► The code can efficiently calculate orientation averaged properties of OA aggregates. ► Interactions among OA spheres can increase the degree of circular polarization.