Biodegradability of all-cellulose composite laminates

The high mechanical properties of single-polymer composites based on degradable non-derivatised cellulose, aka all-cellulose composites, have recently captured the attention of researchers. All-cellulose composites possess the intriguing combination of high strength and biodegradability. However, the biodegradation behaviour of all-cellulose composites has so far not been reported. In this work, soil burial experiments were carried out to compare the biodegradation behaviour of all-cellulose composites with conventional biocomposites in order to investigate the end-of-life disposal of this relatively new class of bio-based composite materials. All-cellulose composites are characterised by exceptional biodegradability with mass losses of up to 73% following a soil burial time of 70 days. An investigation of the mechanisms of biodegradation of all-cellulose composites is undertaken for the first time.