کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
5375419 | 1504292 | 2009 | 6 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Strong-field approximation for high-order above-threshold ionization of randomly oriented diatomic molecules
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
شیمی تئوریک و عملی
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
High-order above-threshold ionization of diatomic molecules by a strong linearly polarized field is considered using the molecular strong-field approximation. Tunneling-rescattering as the mechanism of this ionization gives rise to a novel two-source double-slit interference, which involves the four geometrical paths that are available to an electron, which can be ionized from and rescattered off either of the two centers of the diatomic molecule. For a comparison of this theory with experiments in the absence of molecular alignment, it is necessary to average the theoretical results over the molecular orientation. This paper presents technical details of this averaging procedure. It is shown that, depending on the molecular symmetry, the destructive two-source double-slit interference minima can survive the orientation averaging and can be observed in the angle-resolved electron spectra. This is illustrated on the examples of N2 and O2 molecules. It is also shown that two- and three-dimensional versions of orientation averaging lead to qualitatively similar results.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Chemical Physics - Volume 366, Issues 1â3, 10 December 2009, Pages 85-90
Journal: Chemical Physics - Volume 366, Issues 1â3, 10 December 2009, Pages 85-90
نویسندگان
D.B. MiloÅ¡eviÄ, M. BusuladžiÄ, A. GazibegoviÄ-BusuladžiÄ, W. Becker,