کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
641117 | 1456989 | 2014 | 7 صفحه PDF | دانلود رایگان |
• Fe3O4@LDH@Ag/Ag3PO4 submicrosphere is a novel visible-light photocatalyst.
• The photocatalyst could be easily separated from wastewater for reuse.
• Ag surrounded on Ag3PO4 enhances stability and reusability of Ag3PO4.
• Zn–Cr LDH has high adsorption capacity and facilitates electron–hole separation.
• The photocatalyst shows a high photocatalytic efficiency.
A novel visible-light responsed photocatalyst Fe3O4@LDH@Ag/Ag3PO4 submicrosphere has been successfully prepared by using PO43− intercalated layered double hydroxides (LDH) layers as the intermedium for the formation of Ag3PO4 on the surface of Fe3O4@LDH microspheres. X-ray diffraction (XRD), X-rays photoelectron spectroscopy (XPS), inductively coupled plasma atomic emission spectrum (ICP-AES), high-resolution transmission electron microscopy (HRTEM), field emission and scanning electronic microscope (FESEM) were used to characterize the products. It was found that LDH and Ag/Ag3PO4 layers were successively coated on the Fe3O4 surface. PO43− intercalated LDH played an important role in the formation of Ag/Ag3PO4 nanoparticle on the surface of Fe3O4@LDH microspheres. The studies of photocatalytic degradation on Methylene blue (MB) indicate that the Fe3O4@LDH@Ag/Ag3PO4 photocatalyst showed efficient visible-light-driven photocatalytic activities for degradation of organic pollutants. Furthermore, the photocatalyst could be easily separated from wastewater for reuse by simply applying an external magnetic field. This work provides a facile approach to fabricate novel type of visible-light-responsed photocatalyst for environment treatment.
A novel visible-light responsed photocatalyst Fe3O4@LDH@Ag/Ag3PO4 submicrospheres were successfully prepared by formation of Ag/Ag3PO4 on the surface of Fe3O4@LDH microspheres.Figure optionsDownload as PowerPoint slide
Journal: Separation and Purification Technology - Volume 130, 10 June 2014, Pages 84–90