کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
7128280 1461592 2018 10 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
Nonlinear optical responses of carbon quantum dots anchored on graphene oxide hybrid in solid-state transparent monolithic silica gel glasses
ترجمه فارسی عنوان
پاسخ های غیر خطی نوری نقطه کوانتومی کربن بر روی هیبرید گرافن در عینک ژل سیلیکا یکپارچه شفاف
کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه سایر رشته های مهندسی مهندسی برق و الکترونیک
چکیده انگلیسی
Exploring the nonlinear optical (NLO) response of graphene-based hybrids in solid-state three-dimensional macrostructures is vital to promote the practical development of graphene-based photonic and optoelectronic devices. Here, a solid-state hybrid of ultrafine and well-dispersed carbon quantum dots (CQDs) supported on graphene oxide (GO) was chosen as representative of such materials. The hybrid was introduced into organically modified silica gel glasses using a facile sol-gel wet chemical technique to obtain stable transparent monolithic nanocomposites, and their practical application in nonlinear optics was explored. The NLO performances were investigated by the open-aperture (OA) and closed-aperture (CA) Z-scan techniques in the nanosecond regime using a laser with a wavelength of 532 nm. The as-prepared CQD/GO SiO2 gel glasses displayed completely different NLO behavior from that of a CQD/GO suspension. The NLO performance of CQD/GO significantly improved after incorporation into SiO2 gel glasses because of the more graphitized structure of the CQD/GO hybrid. Both the OA and CA Z-scan patterns suggested that the NLO properties of the CQD/GO suspension combined nonlinear absorption and nonlinear scattering, while the NLO response of the CQD/GO SiO2 gel glasses stemmed primarily from nonlinear absorption and nonlinear refraction. In addition, this is the first report of the third-order nonlinear susceptibility χ(3) of a CQD/GO hybrid doped in solid-state gel glasses. The present results therefore demonstrate the feasibility and versatility of CQD/GO silica gel glasses, a promising new class of highly efficient NLO materials that can be applied in optical communications, radiofrequency optoelectronics, and all-optical signal processing.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Optics & Laser Technology - Volume 107, November 2018, Pages 281-290
نویسندگان
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