کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
8084867 | 1521747 | 2016 | 5 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Chemical diffusion coefficient calculation of U3+ in LiCl-KCl molten salt
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی انرژی
مهندسی انرژی و فناوری های برق
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چکیده انگلیسی
Self-diffusion coefficient denotes the intrinsic diffusion of elements without the chemical gradient; generally, it is different from the chemical diffusion coefficient that is used in Fick's law. However, the self-diffusion coefficient can be converted to the chemical diffusion coefficient by considering the concentration-dependent activity coefficient of solute. In this study, the multiple time origins method was applied to calculate the self-diffusion coefficient of U3+ in LiCl-KCl eutectic salt at different temperatures and concentrations. The chemical diffusion coefficient was obtained based on the calculated results and thermodynamic theory. Calculated results show that self-diffusion coefficient decreases with concentration however chemical diffusion coefficient indicates to change little initially but appears to increase followed by decrease later within the concentration range of 0-3Â at%.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Progress in Nuclear Energy - Volume 91, August 2016, Pages 170-174
Journal: Progress in Nuclear Energy - Volume 91, August 2016, Pages 170-174
نویسندگان
Wentao Zhou, Jinsuo Zhang,