کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
8147722 | 1524153 | 2018 | 23 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Effect of Sn substitution on the elastic anomalies and phase transition behaviors of antiferroelectric PbHfO3 single crystals studied by Brillouin scattering
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
فیزیک و نجوم
فیزیک ماده چگال
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
The phase transition sequence of a PbHf0.7Sn0.3O3 single crystal was investigated by using Brillouin spectroscopy. The longitudinal acoustic mode showed three distinct changes at â¼370â¯K, â¼455â¯K and â¼495â¯K which corresponded to the antiferroelectric 1 â antiferroelectric 2 â intermediate â paraelectric phase transitions upon heating. The paraelectric phase was characterized by softening acoustic mode, increasing acoustic damping and the appearance of quasielastic central peaks which were observed upon approaching the phase transition temperature. The relaxation times derived from the acoustic mode anomalies and the central peak were consistent with each other and showed a slowing-down behavior. These precursor phenomena were attributed to the polar clusters having broken inversion symmetry. The substitution of Hf with Sn induced a very soft intermediate phase between the paraelectric and the antiferroelectric phases, where the longitudinal acoustic mode exhibited the lowest mode frequency along with substantially high acoustic damping. The transverse acoustic mode, which was observed in the two antiferroelectric phases, did not appear in the intermediate phase. These results indicated that the average symmetry of the intermediate phase may be cubic consisting of fine ferroelastic domains.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Current Applied Physics - Volume 18, Issue 6, June 2018, Pages 642-647
Journal: Current Applied Physics - Volume 18, Issue 6, June 2018, Pages 642-647
نویسندگان
Jung-Taek Hong, Byoung Wan Lee, Jae-Hyeon Ko, Irena Jankowska-Sumara, Maria Podgórna, Andrzej Majchrowski,