High-resolution spectroscopy using interleaved 100 GHz optical frequency comb scanned by phase modulator

A high-resolution spectroscopy technique is proposed with an optical phase modulator combined with an interleaved optical frequency comb. The optical phase modulator and a frequency-locked laser light guarantee a spectral resolution less than 1 MHz on an absolute frequency axis. A wide measurement frequency range was realized using a 25 GHz optical frequency comb lying over a 4 THz frequency region. An extraction of single tooth intensity from the comb was realized by a heterodyne technique with a frequency-tunable laser used as a local oscillator. Also, the 25 GHz optical frequency comb was interleaved to generate four 100-GHz combs for removing the crosstalk from the 25 GHz neighboring sidebands in the teeth. This proposed spectroscopy technique was experimentally demonstrated with a resonator of less than 1 MHz linewidth and a H13C14N gas cell. Thus, a measurement frequency range higher than 4 THz (1530 nm–1560 nm) was confirmed with an effective spectral resolution 100 kHz order. In addition, the characteristics of the proposed system were compared with those of the previous system with a single-sideband (SSB) optical modulator.