Feasibility study of minor actinide transmutation in light water reactors with various Am/Cm separation efficiencies

A study was conducted to evaluate the feasibility of minor actinide (MA) transmutation in light water reactors (LWR). The purpose of this work was to provide a guide for future investigations into MA transmutation in LWR. This work considered the effects of various Am/Cm separation efficiencies as well as homogeneous and heterogeneous MA bearing fuel assemblies. The MA content was introduced into the reactor as mixed oxide plus minor actinide (MOX + MA) fuel. Three Am/Cm separation efficiencies were independently considered: 99.9%, 99.0%, and 90.0%. In order to evaluate the feasibility of MA transmutation, the fuel performance of the various assemblies and core designs, as well as their respective safety related parameters, were calculated. The reduction of the burden of high level waste (HLW) motivated the investigation of MA transmutation. It was found that the MA bearing fuel assemblies and their subsequent core designs were able to perform within the safety limits required as well as achieving similar burnups to a UO2 core. The Am transmutation rates were ∼40% for the homogeneous assemblies and up to 68% for the MA targets in the heterogeneous assemblies after the described burnup, however, there was a significant amount of Cm produced during burnup. This Cm production was due to the more favorable neutron capture reaction over fission for Am in the thermal spectrum. Future work should examine the benefits of Am transmutation at the expense of large Cm production rates.

► Minor actinide transmutation in LWR focusing on Am reduction.
► Evaluated three efficiencies of Am/Cm separations: 99.9%, 99.0%, and 90.0%.
► Evaluated MA bearing fuel assemblies of heterogeneous and homogeneous configurations.
► Achieved Am reductions of approximately 40% (homogeneous) and up to 68% (heterogeneous).
► MA bearing fuel assemblies perform within safety limits.