کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
5437539 | 1398175 | 2017 | 28 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Experimental and theoretical analysis of H and Ti co-doped ZnO transparent conductive films
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی مواد
سرامیک و کامپوزیت
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
Ti-doped ZnO (TZO) films were grown by radio frequency (RF) magnetron sputtering using a Ti-doped ZnO ceramic target in an Ar+H2 atmosphere at room temperature. Both the experimental and theoretical methods were employed to investigate the effect of H in TZO films. As the H2 flow rate increased, the surface morphology changed from pyramid-like features to a crater-like topography and the root-mean-square (RMS) roughness increased. The crystal quality was found to deteriorate at first but subsequently improved at an optimum doping ratio. A resistivity of 7.97Ã10â4 Ω cm and an average transmittance of more than 83% in the 400-1100 nm range were obtained with an optimal H2 flow rate of 1.2 sccm. Results of theoretical calculations show that the H dopant behaves as a shallow donor in the TZO films. The doping position of H is located in a BC ⥠configuration at the center of the Zn-O bond, in which the O atom bonded to a substituted Ti atom parallel to the c axis. The charge carrier bands shifted from Ti 3d and O 2p orbitals in the TZO film to Ti 3d and H 1 s orbitals in H and Ti co-doped ZnO films.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Ceramics International - Volume 43, Issue 7, May 2017, Pages 5396-5402
Journal: Ceramics International - Volume 43, Issue 7, May 2017, Pages 5396-5402
نویسندگان
Yanfeng Wang, Jianmin Song, Wei Zheng, Hailin Pei, Xiaohe Wang, Dan Wang, Guozhen Niu, Qinggong Song, Fu Yang, Jingyu Nan,