کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
577215 | 1453097 | 2013 | 7 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Converting hazardous organics into clean energy using a solar responsive dual photoelectrode photocatalytic fuel cell
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موضوعات مرتبط
مهندسی و علوم پایه
مهندسی شیمی
بهداشت و امنیت شیمی
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چکیده انگلیسی
Direct discharging great quantities of organics into water-body not only causes serious environmental pollution but also wastes energy sources. In this paper, a solar responsive dual photoelectrode photocatalytic fuel cell (PFC2) based on TiO2/Ti photoanode and Cu2O/Cu photocathode was designed for hazardous organics treatment with simultaneous electricity generation. Under solar irradiation, the interior bias voltage produced for the Fermi level difference between photoelectrodes drives photoelectrons of TiO2/Ti photoanode to combine with photoholes of Cu2O/Cu photocathode through external circuit thus generating electricity. In the meantime, organics are decomposed by photoholes remained at TiO2/Ti photoanode. By using various hazardous organics including azo dyes as model pollutants, the PFC showed high converting performance of organics into electricity. For example, in 0.05Â M phenol solution, a short-circuit current density 0.23Â mAÂ cmâ2, open-circuit voltage 0.49Â V, maximum power output 0.36Â 10â4Â WÂ cmâ2 was achieved. On the other hand, removal rate of chroma reached 67%, 87% and 63% in 8Â h for methyl orange, methylene blue, Congo red, respectively.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Journal of Hazardous Materials - Volume 262, 15 November 2013, Pages 304-310
Journal: Journal of Hazardous Materials - Volume 262, 15 November 2013, Pages 304-310
نویسندگان
Jianyong Li, Jinhua Li, Quanpeng Chen, Jing Bai, Baoxue Zhou,