کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
8089821 | 1521952 | 2017 | 18 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Supercritical CO2 injection and residence time in fluid-saturated rocks: Evidence for calcite dissolution and effects on rock integrity
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
علوم زمین و سیارات
فرآیندهای سطح زمین
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چکیده انگلیسی
X-ray tomographic monitoring suggests that scCO2 first displaces the water, leading to an average water saturation of about 70-90%. Then, scCO2 dissolves in the pore brine, leading to a homogeneous decrease by about 3% in water saturation of the sample. As a result, the pore brine acidifies even after 2Â h of exposure only, which leads to calcite dissolution and a significant increase in the brine's concentration in calcium cations. For the samples and most exposure experiments, evidence of calcite dissolution is inferred from the measured physical properties. For the brine-saturated Tuffeau limestone and CIPS sandstone, calcite dissolution leads to significant mechanical weakening. For the brine-saturated Savonnieres limestone, the sample subject to two-hour residence time shows evidence of calcite dissolution, whereas the sample after four-hour residence time does not. Calcite re-precipitation could be the cause of this unexpected response after four hours.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: International Journal of Greenhouse Gas Control - Volume 67, December 2017, Pages 31-48
Journal: International Journal of Greenhouse Gas Control - Volume 67, December 2017, Pages 31-48
نویسندگان
Lucas Pimienta, Lionel Esteban, Joel Sarout, Keyu Liu, Jérémie Dautriat, Claudio Delle Piane, Michael B. Clennell,